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- W3120169884 endingPage "417" @default.
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- W3120169884 abstract "Anionic NHC ligands recently developed in our group, derived from N-iminoimidazolium ylides, were used to synthesize NHC-iridium(III) complexes. Their catalytic activities were evaluated in the amine alkylation of anilines using borrowing hydrogen catalysis. The high-yielding synthesis of a small library of complexes allowed a rapid screening of the ideal steric bulk of the NHC unit and basicity of the anionic tether for the investigated model reaction. A bulky aromatic N group on the imidazolidene moiety is required to achieve high catalytic activity, and the latter is proportional to the basicity of the anionic group. A selected substrate scope of the reaction was performed, providing fair to excellent yields of the desired alkylated anilines." @default.
- W3120169884 created "2021-01-18" @default.
- W3120169884 creator A5028392243 @default.
- W3120169884 creator A5055522735 @default.
- W3120169884 date "2021-01-13" @default.
- W3120169884 modified "2023-10-16" @default.
- W3120169884 title "Synthesis of NHC-Iridium(III) Complexes Based on<i>N</i>-Iminoimidazolium Ylides and Their Use for the Amine Alkylation by Borrowing Hydrogen Catalysis" @default.
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- W3120169884 doi "https://doi.org/10.1021/acs.organomet.0c00726" @default.
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