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- W3120235026 abstract "The discovery of granular adsorbents for the capture of volatile organic compounds (VOCs) from humid air and rapid regeneration at low temperature is still a challenge. Here we reported formation of a granular Al-based metal organic gel, CAU-3-NH2(gel), by adjusting heating up time in the synthesis procedure. The water and thermal stable xerogel shows high surface area (1964 m2/g) and adsorption capacity for VOCs (uptakes of toluene and hexanal reach 4.5 and 3.85 mmol/g at P/P0 = 0.1, respectively). Dynamic adsorption experiments further conformed its outstanding adsorption performance for toluene under 50% RH, higher than that of commercial adsorbents and widely studied MOFs including BPL activated carbon, ZSM-5, zeolite 13X, XAD-16, MIL-101(Cr), CAU-1 and ZIF-8. Under the mass space velocity of 12,000 mL/g.h, CAU-3-NH2(gel) kept 99.95% removal ratio of low concentration toluene (100 ppm) over 12 h in 3 cycles at 298 K. Furthermore, desorption experiments show its excellent regenerability under mild temperature (328 K and 358 K). The interaction of toluene-framework and adsorption process are investigated by using Grand Canonical Monte Carlo (GCMC) simulations." @default.
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- W3120235026 date "2021-06-01" @default.
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- W3120235026 title "Energy-efficient capture of volatile organic compounds from humid air by granular metal organic gel" @default.
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- W3120235026 doi "https://doi.org/10.1016/j.jhazmat.2021.125057" @default.
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