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• W3121030428 abstract "Fabrication of 3d metal-based core@shell nanocatalysts with engineered Pt-surfaces provides an effective approach for improving the catalytic performance. The challenges in such preparation include shape control of the 3d metallic cores and thickness control of the Pt-based shells. Herein, we report a colloidal seed-mediated method to prepare octahedral CuNi@Pt-Cu core@shell nanocrystals using CuNi octahedral cores as the template. By precisely controlling the synthesis conditions including the deposition rate and diffusion rate of the shell-formation through tuning the capping ligand, reaction temperature, and heating rate, uniform Pt-based shells can be achieved with a thickness of <1 nm. The resultant carbon-supported CuNi@Pt-Cu core@shell nano-octahedra showed superior activity in electrochemical methanol oxidation reaction (MOR) compared with the commercial Pt/C catalysts and carbon-supported CuNi@Pt-Cu nano-polyhedron counterparts." @default.
• W3121030428 created "2021-01-18" @default.
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• W3121030428 date "2021-02-25" @default.
• W3121030428 modified "2023-10-11" @default.
• W3121030428 title "Synthesis of Core@Shell Cu‐Ni@Pt‐Cu Nano‐Octahedra and Their Improved MOR Activity" @default.
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• W3121030428 doi "https://doi.org/10.1002/anie.202014144" @default.
• W3121030428 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33438300" @default.
• W3121030428 hasPublicationYear "2021" @default.
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