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• W3121082641 startingPage "102056" @default.
• W3121082641 abstract "Methanol dehydrogenation is an efficient way to produce syngas with high quality. The current efficiency of sunlight-driven methanol dehydrogenation is poor, which is limited by the lack of excellent catalysts and effective methods to convert sunlight into chemicals. Here, we show that atomically substitutional Pt-doped in CeO2 nanosheets (Pts-CeO2) exhibit excellent methanol dehydrogenation activity with 500-hr level catalytic stability, 11 times higher than that of Pt nanoparticles/CeO2. Further, we introduce a photothermal conversion device to heat Pts-CeO2 up to 299°C under 1 sun irradiation owning to efficient full sunlight absorption and low heat dissipation, thus achieving an extraordinarily high methanol dehydrogenation performance with a 481.1 mmol g−1 h−1 of H2 production rate and a high solar-to-hydrogen (STH) efficiency of 32.9%. Our method represents another progress for ambient sunlight-driven stable and active methanol dehydrogenation technology." @default.
• W3121082641 created "2021-01-18" @default.
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• W3121082641 date "2021-02-01" @default.
• W3121082641 modified "2023-10-14" @default.
• W3121082641 title "Ambient sunlight-driven photothermal methanol dehydrogenation for syngas production with 32.9 % solar-to-hydrogen conversion efficiency" @default.
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• W3121082641 doi "https://doi.org/10.1016/j.isci.2021.102056" @default.
• W3121082641 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7841357" @default.
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