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• W3121641898 endingPage "2006577" @default.
• W3121641898 startingPage "2006577" @default.
• W3121641898 abstract "The development of all-solid-state Li metal batteries (ASSLMBs) has attracted significant attention due to their potential to maximize energy density and improved safety compared to the conventional liquid-electrolyte-based Li-ion batteries. However, it is very challenging to fabricate an ideal solid-state electrolyte (SSE) that simultaneously possesses high ionic conductivity, excellent air-stability, and good Li metal compatibility. Herein, a new glass-ceramic Li3.2P0.8Sn0.2S4 (gc-Li3.2P0.8Sn0.2S4) SSE is synthesized to satisfy the aforementioned requirements, enabling high-performance ASSLMBs at room temperature (RT). Compared with the conventional Li3PS4 glass-ceramics, the present gc-Li3.2P0.8Sn0.2S4 SSE with 12% amorphous content has an enlarged unit cell and a high Li+ ion concentration, which leads to 6.2-times higher ionic conductivity (1.21 × 10−3 S cm−1 at RT) after a simple cold sintering process. The (P/Sn)S4 tetrahedron inside the gc-Li3.2P0.8Sn0.2S4 SSE is verified to show a strong resistance toward reaction with H2O in 5%-humidity air, demonstrating excellent air-stability. Moreover, the gc-Li3.2P0.8Sn0.2S4 SSE triggers the formation of Li–Sn alloys at the Li/SSE interface, serving as an essential component to stabilize the interface and deliver good electrochemical performance in both symmetric and full cells. The discovery of this gc-Li3.2P0.8Sn0.2S4 superionic conductor enriches the choice of advanced SSEs and accelerates the commercialization of ASSLMBs." @default.
• W3121641898 created "2021-02-01" @default.
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• W3121641898 date "2021-01-20" @default.
• W3121641898 modified "2023-10-06" @default.
• W3121641898 title "An Air‐Stable and Li‐Metal‐Compatible Glass‐Ceramic Electrolyte enabling High‐Performance All‐Solid‐State Li Metal Batteries" @default.
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• W3121641898 doi "https://doi.org/10.1002/adma.202006577" @default.
• W3121641898 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33470466" @default.
• W3121641898 hasPublicationYear "2021" @default.
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