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- W3122023508 abstract "Owing to the urgent demand for CO2 emission and the increasing need for the utilization of waste glycerol from biodiesel production, cobalt-based zeolitic imidazolate framework-67 (ZIF-67) was prepared as a catalyst for the carboxylation of glycerol to glycerol carbonate under different reaction conditions. ZIF-67 exhibited high crystallinity, a high specific surface area of ~1250 m2 g−1, promising thermal stability with a weight loss of ~10% above 400 °C, facile ligand-to-metal electron transition, and numerous Lewis basic sites, indicating its high catalytic activity. The conversion, yield, and selectivity achieved with ZIF-67 were 32, 29, and 92%, respectively, at reaction temperature and duration of 210 °C for 12 h, respectively. The catalytic gas–liquid reaction followed third-order kinetics. This is the first study to elucidate the reaction kinetics of glycerol carboxylation using ZIF-67 as a catalyst and to highlight the potential of ZIF-67 as a functional catalyst for CO2–glycerol conversion." @default.
- W3122023508 created "2021-02-01" @default.
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- W3122023508 date "2021-05-01" @default.
- W3122023508 modified "2023-10-16" @default.
- W3122023508 title "Production of glycerol carbonate from carboxylation of glycerol with CO2 using ZIF-67 as a catalyst" @default.
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- W3122023508 doi "https://doi.org/10.1016/j.ces.2021.116451" @default.
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