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• W3122156765 startingPage "7669" @default.
• W3122156765 abstract "Anilines are some of the most used class of substrates for application in photoinduced electron transfer. N,N-Dialkyl-derivatives enable radical generation α to the N-atom by oxidation followed by deprotonation. This approach is however elusive to monosubstituted anilines owing to fast back-electron transfer (BET). Here we demonstrate that BET can be minimised by using photoredox catalysis in the presence of an exogenous alkylamine. This approach synergistically aids aniline SET oxidation and then accelerates the following deprotonation. In this way, the generation of α-anilinoalkyl radicals is now possible and these species can be used in a general sense to achieve divergent sp3 C−H functionalization." @default.
• W3122156765 created "2021-02-01" @default.
• W3122156765 creator A5050256902 @default.
• W3122156765 creator A5071065862 @default.
• W3122156765 date "2021-03-03" @default.
• W3122156765 modified "2023-10-03" @default.
• W3122156765 title "Minimization of Back‐Electron Transfer Enables the Elusive sp ³ C−H Functionalization of Secondary Anilines" @default.
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• W3122156765 doi "https://doi.org/10.1002/anie.202100051" @default.
• W3122156765 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/8048505" @default.
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• W3122156765 hasPublicationYear "2021" @default.
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