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- W3123548436 abstract "Abstract A [Fe‐S‐Fe] subunit with a single sulfide bridging two low‐coordinate iron ions is the supposed active site of the iron‐molybdenum co‐factor (FeMoco) of nitrogenase. Here we report a dinuclear monosulfido bridged diiron(II) complex with a similar complex geometry that can be oxidized stepwise to diiron(II/III) and diiron(III/III) complexes while retaining the [Fe‐S‐Fe] core. The series of complexes has been characterized crystallographically, and electronic structures have been studied using, inter alia, 57 Fe Mössbauer spectroscopy and SQUID magnetometry. Further, cleavage of the [Fe‐S‐Fe] unit by CS 2 is presented." @default.
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- W3123548436 date "2021-03-05" @default.
- W3123548436 modified "2023-10-15" @default.
- W3123548436 title "A Molecular Low‐Coordinate [Fe‐S‐Fe] Unit in Three Oxidation States" @default.
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- W3123548436 doi "https://doi.org/10.1002/chem.202100336" @default.
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