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• W3124001503 abstract "Designing highly active transition-metal-based electrocatalysts for energy-saving electrochemical hydrogen evolution coupled with hydrazine oxidation possesses more economic prospects. However, the lack of bifunctional electrocatalysts and the absence of intrinsic structure-property relationship research consisting of adsorption configurations and dehydrogenation behavior of N2H4 molecules still hinder the development. Now, a V-doped Ni3N nanosheet self-supported on Ni foam (V-Ni3N NS) is reported, which presents excellent bifunctional electrocatalytic performance toward both hydrazine oxidation reaction (HzOR) and hydrogen evolution reaction (HER). The resultant V-Ni3N NS achieves an ultralow working potential of 2 mV and a small overpotential of 70 mV at 10 mA cm-2 in alkaline solution for HzOR and HER, respectively. Density functional theory calculations reveal that the vanadium substitution could effectively modulate the electronic structure of Ni3N, therefore facilitating the adsorption/desorption behavior of H* for HER, as well as boosting the dehydrogenation kinetics for HzOR." @default.
• W3124001503 created "2021-02-01" @default.
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• W3124001503 date "2021-01-19" @default.
• W3124001503 modified "2023-10-18" @default.
• W3124001503 title "Vanadium Substitution Steering Reaction Kinetics Acceleration for Ni₃N Nanosheets Endows Exceptionally Energy-Saving Hydrogen Evolution Coupled with Hydrazine Oxidation" @default.
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• W3124001503 doi "https://doi.org/10.1021/acsami.0c18684" @default.
• W3124001503 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33464037" @default.
• W3124001503 hasPublicationYear "2021" @default.
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