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- W3124552264 abstract "Inadequate photogenerated carriers’ separation is deemed to be the major obstacles for improving photocatalytic H2 evolution. Here, we designed distinctive Ni2P/porous g-C3N4/Cd0.5Zn0.5Se-diethylenetriamine (Ni2P/pg-C3N4/Cd0.5Zn0.5Se-D) nanojunction via an in-situ solvothermal synthesis. The cooperative effect of Cd0.5Zn0.5Se-D and Ni2P can extend the visible light absorption for pg-C3N4. As a result, the ternary Ni2P/pg-C3N4/Cd0.5Zn0.5Se-D composite exhibits high-performance H2 evolution rate of 12627 μmol g−1 h−1 using solar light, being almost 105.23 and 2.59 folds higher than those observed over Ni2P/pg-C3N4 and pg-C3N4/Cd0.5Zn0.5Se-D composite, severally. The possible mechanism is assumed that the formation of the novel Ni2P modified step-scheme (S-scheme) pg-C3N4/Cd0.5Zn0.5Se-D heterojunction which manipulated highly efficient spatial separation and directional migration of photocarriers. Moreover, DFT calculations have been performed to uncover the process of the charge transport. This work concentrates on the profound part of noble-metal-free decorated S-scheme photocatalytic system in water splitting." @default.
- W3124552264 created "2021-02-01" @default.
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- W3124552264 creator A5078874545 @default.
- W3124552264 date "2021-05-01" @default.
- W3124552264 modified "2023-09-27" @default.
- W3124552264 title "Insight into the synergy of amine-modified S-scheme Cd0.5Zn0.5Se/porous g-C3N4 and noble-metal-free Ni2P for boosting photocatalytic hydrogen generation" @default.
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- W3124552264 doi "https://doi.org/10.1016/j.ceramint.2021.01.207" @default.
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