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• W3124565890 abstract "Abstract Vibrational sum-frequency generation (vSFG) spectroscopy allows the study of the structure and dynamics of interfacial systems. In the present work, we provide a simple recipe, based on a narrowband IR pump and broadband vSFG probe technique, to computationally obtain the two-dimensional vSFG spectrum of water molecules at the air–water interface. Using this technique, to study the time-dependent spectral evolution of hydrogen-bonded and free water molecules, we demonstrate that at the interface, the vibrational spectral dynamics of the free OH bond is faster than that of the bonded OH mode." @default.
• W3124565890 created "2021-02-01" @default.
• W3124565890 creator A5076340488 @default.
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• W3124565890 date "2021-01-28" @default.
• W3124565890 modified "2023-10-01" @default.
• W3124565890 title "Hydrogen bond dynamics of interfacial water molecules revealed from two-dimensional vibrational sum-frequency generation spectroscopy" @default.
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• W3124565890 doi "https://doi.org/10.1038/s41598-021-81635-4" @default.
• W3124565890 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7844302" @default.
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• W3124565890 hasPublicationYear "2021" @default.
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