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• W3124587588 abstract "High electron affinity (EA) molecules p-type dope low ionization energy (IE) polymers, resulting in an equilibrium doping level based on the energetic driving force (IE-EA), reorganization energy, and dopant concentration. Anion exchange doping (AED) is a process whereby the dopant anion is exchanged with a stable ion from an electrolyte. We show that the AED level can be predicted using an isotherm equilibrium model. The exchange of the dopant anion (FeCl3–) for a bis(trifluoromethanesulfonamide) (TFSI–) anion in the polymers poly(3-hexylthiophene-2,5-diyl) (P3HT) and poly[3-(2,2-bithien-5-yl)-2,5-bis(2-hexyldecyl)-2,5-dihydropyrrolo[3,4-c]pyrrole-1,4-dione-6,5-diyl] (PDPP-2T) highlights two cases in which the process is nonspontaneous and spontaneous, respectively. For P3HT, FeCl3 provides a high doping level but an unstable counterion, so exchange results in an air stable counterion with a marginal increase in doping. For PDPP-2T, FeCl3 is a weak dopant, but the exchange of FeCl3– for TFSI– is spontaneous, so the doping level increases by >10× with AED." @default.
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• W3124587588 date "2021-01-26" @default.
• W3124587588 modified "2023-10-14" @default.
• W3124587588 title "Anion Exchange Doping: Tuning Equilibrium to Increase Doping Efficiency in Semiconducting Polymers" @default.
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• W3124587588 doi "https://doi.org/10.1021/acs.jpclett.0c03620" @default.
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