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• W3124844103 abstract "Abstract The [Fe II (C 6 F 5 Tp) 2 ] spin‐crossover complex is an atypical molecular switch, which can be converted upon annealing between two archetypal spin‐crossover behaviours: from an extremely gradual spin‐crossover to a broad hysteretic spin‐transition (of ca. 65 K). The hysteresis shows an uncommon “rounded shape” that is reproducible upon cycling temperature. In depth structural studies reveal a first crystal phase transition, which occurs upon melting and recrystallizing at high temperature. This first irreversible transition is associated with a radical change in the crystal packing. More importantly, the “rounded and broad” hysteretic transition is shown to occur in a non‐cooperative SCO system and is associated with the occurrence of a symmetry‐breaking phase transition that appears when roughly ca. 50 % of the SCO complexes are switched." @default.
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• W3124844103 date "2021-03-05" @default.
• W3124844103 modified "2023-10-05" @default.
• W3124844103 title "The Atypical Hysteresis of [Fe(C₆F₅Tp)₂]: Overlay of Spin‐Crossovers and Symmetry‐Breaking Phase Transition" @default.
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• W3124844103 doi "https://doi.org/10.1002/anie.202015994" @default.
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