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• W3125137194 endingPage "1287" @default.
• W3125137194 startingPage "1281" @default.
• W3125137194 abstract "Main observation and conclusion We report herein a Re‐based tricarbonyl catalyst [ fac ‐Re(L1)(CO) 3 Cl] (Re1) bearing a spiro center and a phenol group as a local proton source in the second coordination sphere. Due to the large steric spiro group, dimerization of one‐electron reduced species was completely eliminated, improving the stability of Re1. Simultaneously, the phenol group in the second coordination sphere improves the formation of an H‐bonding chain that promotes the protonation of CO 2 reduction intermediates, boosting the electrocatalytic CO 2 reduction activity of Re1. Mechanistic studies reveal that the doubly reduced complex Re1b is active for CO 2 addition." @default.
• W3125137194 created "2021-02-01" @default.
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• W3125137194 date "2021-04-28" @default.
• W3125137194 modified "2023-10-18" @default.
• W3125137194 title "Electrocatalytic<scp>CO₂</scp>Reduction with<scp>Re‐Based</scp>Spiro Bipyridine Complexes: Effects of the Local Proton in the Second Coordination Sphere^†" @default.
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• W3125137194 doi "https://doi.org/10.1002/cjoc.202000667" @default.
• W3125137194 hasPublicationYear "2021" @default.
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