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• W3125639079 abstract "Active species were introduced into MOFs to prepare multifunctional fluorescent probes by a stepwise postsynthetic modulation strategy. First, two-dimensional HPU-16 (HPU = Henan Polytechnic University; HPU-16 = Zn(L)2(H2O); HL = 2-(5-pyridin-4-yl-5H-[1,2,4]triazol-3-yl)-pyrazine) was transformed into three-dimensional HPU-17 ({Zn3(L)2(btc)2(H2O)}n) through a crystal dissolution–recrystallization process. Second, linker replacement was used to introduce −NH2 into the HPU-17 to generate functional NH2-HPU-17 via a single-crystal to single-crystal transformation. The functional amino groups caused NH2-HPU-17 to show a significant response to ClO–. Because of the interaction of amino groups and ClO–, the fluorescence of NH2-HPU-17 gradually changed from blue to yellow-green. More interestingly, NH2-HPU-17 could encapsulate Tb3+ and sensitize the visible-emitting characteristic fluorescence of Tb3+ in aqueous solution. Then, newly generated Tb3+@NH2-HPU-17 could serve as an effective probe for the determination of DPA. This work paves a new way for the design and modulation of ratiometric fluorescence probes for the selective and sensitive detection of special molecules." @default.
• W3125639079 created "2021-02-01" @default.
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• W3125639079 date "2021-01-26" @default.
• W3125639079 modified "2023-10-18" @default.
• W3125639079 title "Postsynthesis Strategy of Functional Zn-MOF Sensors for the Detection of ClO^– and DPA" @default.
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• W3125639079 doi "https://doi.org/10.1021/acs.inorgchem.0c03468" @default.
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• W3125639079 hasPublicationYear "2021" @default.
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