Matches in SemOpenAlex for { <https://semopenalex.org/work/W3126128924> ?p ?o ?g. }
- W3126128924 abstract "Transitions metal dichalcogenides (TMDs) are direct semiconductors in the atomic monolayer (ML) limit with fascinating optical and spin-valley properties. The strong optical absorption of up to 20 % for a single ML is governed by excitons, electron-hole pairs bound by Coulomb attraction. Excited exciton states in MoSe$_2$ and MoTe$_2$ monolayers have so far been elusive due to their low oscillator strength and strong inhomogeneous broadening. Here we show that encapsulation in hexagonal boron nitride results in emission line width of the A:1$s$ exciton below 1.5 meV and 3 meV in our MoSe$_2$ and MoTe$_2$ monolayer samples, respectively. This allows us to investigate the excited exciton states by photoluminescence upconversion spectroscopy for both monolayer materials. The excitation laser is tuned into resonance with the A:1$s$ transition and we observe emission of excited exciton states up to 200 meV above the laser energy. We demonstrate bias control of the efficiency of this non-linear optical process. At the origin of upconversion our model calculations suggest an exciton-exciton (Auger) scattering mechanism specific to TMD MLs involving an excited conduction band thus generating high energy excitons with small wave-vectors. The optical transitions are further investigated by white light reflectivity, photoluminescence excitation and resonant Raman scattering confirming their origin as excited excitonic states in monolayer thin semiconductors." @default.
- W3126128924 created "2021-02-01" @default.
- W3126128924 creator A5008639157 @default.
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- W3126128924 creator A5041573207 @default.
- W3126128924 creator A5045096283 @default.
- W3126128924 creator A5045247857 @default.
- W3126128924 creator A5057268563 @default.
- W3126128924 creator A5066772150 @default.
- W3126128924 creator A5067326259 @default.
- W3126128924 creator A5067479351 @default.
- W3126128924 creator A5069535863 @default.
- W3126128924 creator A5089325282 @default.
- W3126128924 date "2018-09-18" @default.
- W3126128924 modified "2023-10-16" @default.
- W3126128924 title "Exciton States in Monolayer <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi>MoSe</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> and <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi>MoTe</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> Probed by Upconversion Spectroscopy" @default.
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