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- W3126832774 abstract "Abstract It is crucial and desirable to develop green and high-efficient strategies to regulate solid-state structures and their related material properties. However, relative to solution, it is more difficult to break and generate chemical bonds in solid states. In this work, a rubbing-induced photoluminescence on the solid states of ortho-pyridinil phenol family was achieved. This rubbing response relied on an accurately designed topochemical tautomerism, where a negative charge, exactly provided by the triboelectric effect of a rubber, can induce a proton transfer in a double H-bonded dimeric structure. This process instantaneously led to a bright-form tautomer that can be stabilized in the solid-state settings, leading to an up to over 450-fold increase of the fluorescent quantum yield of the materials. The property can be repeatedly used due to the reversibility of the tautomerism, enabling encrypted applications. Moreover, a further modification to the structure can be accomplished to achieve different properties, opening up more possibilities for the design of new-generation smart materials." @default.
- W3126832774 created "2021-02-15" @default.
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- W3126832774 date "2021-02-10" @default.
- W3126832774 modified "2023-10-01" @default.
- W3126832774 title "Lighting up solid states using a rubber" @default.
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- W3126832774 doi "https://doi.org/10.1038/s41467-021-21253-w" @default.
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