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- W3126973792 abstract "This article reveals that molybdenum (Mo) heteroatoms isomorphously substituted decatungstates (Mo–DTs) can be conveniently synthesized via copolymerization of tungstate and molybdate in acidic solution. A series of characterizations support that the incorporated Mo heteroatoms play crucial roles in improving the redox capacity and visible light harvesting efficiency of Mo–DTs, especially the photo-excited probability and lifetimes, so that the novel Mo–DTs exhibit a remarkably enhanced photo-catalytic efficiency in the visible-light-triggered selective oxidation of inert hydrocarbons by O2 under mild conditions. In the photo-oxidation of cyclohexane under continuous visible light irradiation for 30 h, the best 1 % Mo–DT can achieve 44.8 % conversion and 89.7 % cyclohexanone selectivity in the presence of 2 M HCl, and the regenerated catalyst after simple hydrothermal treatment has excellent reusability. This is the first successful example of incorporating Mo atoms into the skeleton of non-lacunary DTs, which has special significance for expanding the application of DTs in visible-light-catalysis." @default.
- W3126973792 created "2021-02-15" @default.
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- W3126973792 date "2021-03-03" @default.
- W3126973792 modified "2023-09-22" @default.
- W3126973792 title "Molybdenum Isomorphously Substituted Decatungstates as Robust and Renewable Photocatalysts for Visible Light‐Driven Oxidation of Hydrocarbons by Molecular Oxygen" @default.
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- W3126973792 doi "https://doi.org/10.1002/cctc.202002037" @default.
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