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- W3128082029 abstract "Abstract The low effectiveness factor of catalyst pellet caused by high internal diffusion limitation is a common issue in fixed‐bed reactor. Nevertheless, hierarchical structured catalyst provides a promising solution for the contradiction between reaction activity and diffusion efficiency in large catalyst pellets. Herein, we studied the effect of pore structure parameters of the meso‐macroporous catalyst on Fischer–Tropsch synthesis performances through experiment and pellet scale reaction–diffusion simulation. The pellet simulation firstly elucidated the reason for the significant improvement on activity and product selectivity for the meso‐macroporous catalyst observed in our experiment. Further optimization via pellet simulation indicated the critical influences of wax filling degree and that the perfect matching between reaction and mass transfer rates by increasing macropore size and adjusting porosity within pellet enables the C 5+ space–time yield to the maximum. This work could provide a theoretical guideline for the engineering design of the hierarchical structured catalyst pellet." @default.
- W3128082029 created "2021-02-15" @default.
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- W3128082029 date "2021-02-15" @default.
- W3128082029 modified "2023-10-18" @default.
- W3128082029 title "Mass transfer advantage of hierarchical structured cobalt‐based catalyst pellet for <scp>Fischer–Tropsch</scp> synthesis" @default.
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- W3128082029 doi "https://doi.org/10.1002/aic.17226" @default.
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