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• W3128662647 startingPage "100663" @default.
• W3128662647 abstract "The practical application of lithium (Li) metal anode has been greatly hampered by irregular growth of Li dendrites and the volume expansion during the cycle. Constructing a three-dimensional lithiophilic porous framework is regarded as an effective solution. Here, using a CuO nanocluster arrays–decorated carbon fiber cloth (CuO-NC@CFC) to prestore Li via molten infusion has been testified to effectively resolve these bottlenecks. Impressively, after a violent melt-infusion process, the constructed nanostructures can be maintained and transformed into Cu/Li 2 O nanocluster arrays, together with highly conductive carbon fiber cloth, provide fast charge transport during Li stripping/plating process. As demonstrated by finite element simulations and experimental evidence, the formed Cu/Li 2 O nanocluster arrays not only redistribute Li + flux and reduce local current density but also serve as Li nucleation sites. Consequently, the as-acquired Li/Cu-NC@CFC electrodes could significantly buffer volume fluctuation and regulate Li deposition behavior, exhibiting an ultrastable and ultralong lifespan (400 h at 5 mA/cm 2 with 1 mAh/cm 2 Li and 800 h at 5 mA/cm 2 with 5 mAh/cm 2 Li in symmetric cells). When coupled with LiFePO 4 , the Li/Cu-NC@CFC electrode could deliver a high capacity of 110.3 mAh/g after 500 cycles at 2 C. • The Li/Cu-NC@CFC electrode was prepared via a facile molten lithium infusion strategy. • The Cu/Li 2 O nanocluster arrays reduce local current density and regulate Li + flux. • The carbon fiber cloth alleviates the volume change and ensures a fast charge transfer kinetics. • The Li/Cu-NC@CFC electrodes exhibit impressive performance in cycling tests." @default.
• W3128662647 created "2021-02-15" @default.
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• W3128662647 date "2021-06-01" @default.
• W3128662647 modified "2023-10-14" @default.
• W3128662647 title "Rationally optimized carbon fiber cloth as lithiophilic host for highly stable Li metal anodes" @default.
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• W3128662647 doi "https://doi.org/10.1016/j.mtener.2021.100663" @default.
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