Matches in SemOpenAlex for { <https://semopenalex.org/work/W3128663453> ?p ?o ?g. }
- W3128663453 endingPage "100090" @default.
- W3128663453 startingPage "100090" @default.
- W3128663453 abstract "•OSCs are a promising technology to transform the solar energy to electricity•This article reports an efficient TCCT photovoltaic material through subtle side-chain modification•The TCCT property enables 13% efficiency with FF reaching 70% in 470 nm thick-film photovoltaics To clearly show how important the impact of side chains on organic solar cells (OSCs) is, we designed three acceptors IDIC-CxPh (x = 4, 5, or 6) via subtle side-chain regulation. Despite this small change, significant distinctions were detected. IDIC-C4Ph devices achieve an optimal efficiency of 13.94% under thermal annealing, but thermal-assistant solvent-vapor annealing hugely suppresses the efficiencies to 10%. However, the C6Ph side chain endows extremely disordered stacking orientations, generating moderate efficiencies of ~12.50%. Excitingly, the IDIC-C5Ph affords an unexpected two-channel π-π charge transport (TCCT) property, boosting the fill factor (FF) by up to 80.02% and efficiency to 14.56%, ranking the best among five-ring fused-ladder-type acceptors. Impressively, the special TCCT behavior of IDIC-C5Ph enables 470 nm thick-film OSC with a high FF of up to 70.12% and efficiency of 13.01%, demonstrating the great promise in fabricating large-scale OSCs. To clearly show how important the impact of side chains on organic solar cells (OSCs) is, we designed three acceptors IDIC-CxPh (x = 4, 5, or 6) via subtle side-chain regulation. Despite this small change, significant distinctions were detected. IDIC-C4Ph devices achieve an optimal efficiency of 13.94% under thermal annealing, but thermal-assistant solvent-vapor annealing hugely suppresses the efficiencies to 10%. However, the C6Ph side chain endows extremely disordered stacking orientations, generating moderate efficiencies of ~12.50%. Excitingly, the IDIC-C5Ph affords an unexpected two-channel π-π charge transport (TCCT) property, boosting the fill factor (FF) by up to 80.02% and efficiency to 14.56%, ranking the best among five-ring fused-ladder-type acceptors. Impressively, the special TCCT behavior of IDIC-C5Ph enables 470 nm thick-film OSC with a high FF of up to 70.12% and efficiency of 13.01%, demonstrating the great promise in fabricating large-scale OSCs." @default.
- W3128663453 created "2021-02-15" @default.
- W3128663453 creator A5000576799 @default.
- W3128663453 creator A5015065738 @default.
- W3128663453 creator A5025524686 @default.
- W3128663453 creator A5034427968 @default.
- W3128663453 creator A5053738480 @default.
- W3128663453 creator A5063642659 @default.
- W3128663453 creator A5073084208 @default.
- W3128663453 creator A5083377250 @default.
- W3128663453 creator A5086925064 @default.
- W3128663453 creator A5091078676 @default.
- W3128663453 creator A5091527569 @default.
- W3128663453 date "2021-02-01" @default.
- W3128663453 modified "2023-10-17" @default.
- W3128663453 title "Subtle Side Chain Triggers Unexpected Two-Channel Charge Transport Property Enabling 80% Fill Factors and Efficient Thick-Film Organic Photovoltaics" @default.
- W3128663453 cites W1988567331 @default.
- W3128663453 cites W2025120535 @default.
- W3128663453 cites W2067472967 @default.
- W3128663453 cites W2071134066 @default.
- W3128663453 cites W2079578273 @default.
- W3128663453 cites W2082019533 @default.
- W3128663453 cites W2124474427 @default.
- W3128663453 cites W2140762509 @default.
- W3128663453 cites W2643458945 @default.
- W3128663453 cites W2752133241 @default.
- W3128663453 cites W2765398234 @default.
- W3128663453 cites W2769916051 @default.
- W3128663453 cites W2772390981 @default.
- W3128663453 cites W2774538686 @default.
- W3128663453 cites W2782930971 @default.
- W3128663453 cites W2783974197 @default.
- W3128663453 cites W2804473947 @default.
- W3128663453 cites W2804841348 @default.
- W3128663453 cites W2807774288 @default.
- W3128663453 cites W2809110541 @default.
- W3128663453 cites W2874021137 @default.
- W3128663453 cites W2889452188 @default.
- W3128663453 cites W2909990379 @default.
- W3128663453 cites W2912017373 @default.
- W3128663453 cites W2912563757 @default.
- W3128663453 cites W2933655516 @default.
- W3128663453 cites W2937791499 @default.
- W3128663453 cites W2948438814 @default.
- W3128663453 cites W2949529830 @default.
- W3128663453 cites W2958853574 @default.
- W3128663453 cites W2965610870 @default.
- W3128663453 cites W2968730424 @default.
- W3128663453 cites W2978277691 @default.
- W3128663453 cites W2981412106 @default.
- W3128663453 cites W2999590263 @default.
- W3128663453 cites W3006781409 @default.
- W3128663453 cites W3011388529 @default.
- W3128663453 cites W3013363765 @default.
- W3128663453 cites W3016117235 @default.
- W3128663453 cites W3022108908 @default.
- W3128663453 cites W3028691354 @default.
- W3128663453 cites W3028938884 @default.
- W3128663453 cites W3043311860 @default.
- W3128663453 cites W3043334510 @default.
- W3128663453 cites W3092176414 @default.
- W3128663453 doi "https://doi.org/10.1016/j.xinn.2021.100090" @default.
- W3128663453 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/8454635" @default.
- W3128663453 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34557744" @default.
- W3128663453 hasPublicationYear "2021" @default.
- W3128663453 type Work @default.
- W3128663453 sameAs 3128663453 @default.
- W3128663453 citedByCount "38" @default.
- W3128663453 countsByYear W31286634532021 @default.
- W3128663453 countsByYear W31286634532022 @default.
- W3128663453 countsByYear W31286634532023 @default.
- W3128663453 crossrefType "journal-article" @default.
- W3128663453 hasAuthorship W3128663453A5000576799 @default.
- W3128663453 hasAuthorship W3128663453A5015065738 @default.
- W3128663453 hasAuthorship W3128663453A5025524686 @default.
- W3128663453 hasAuthorship W3128663453A5034427968 @default.
- W3128663453 hasAuthorship W3128663453A5053738480 @default.
- W3128663453 hasAuthorship W3128663453A5063642659 @default.
- W3128663453 hasAuthorship W3128663453A5073084208 @default.
- W3128663453 hasAuthorship W3128663453A5083377250 @default.
- W3128663453 hasAuthorship W3128663453A5086925064 @default.
- W3128663453 hasAuthorship W3128663453A5091078676 @default.
- W3128663453 hasAuthorship W3128663453A5091527569 @default.
- W3128663453 hasBestOaLocation W31286634531 @default.
- W3128663453 hasConcept C119599485 @default.
- W3128663453 hasConcept C127413603 @default.
- W3128663453 hasConcept C159985019 @default.
- W3128663453 hasConcept C178790620 @default.
- W3128663453 hasConcept C185592680 @default.
- W3128663453 hasConcept C192562407 @default.
- W3128663453 hasConcept C204921945 @default.
- W3128663453 hasConcept C2777855556 @default.
- W3128663453 hasConcept C33347731 @default.
- W3128663453 hasConcept C41291067 @default.
- W3128663453 hasConcept C49040817 @default.
- W3128663453 hasConcept C521977710 @default.
- W3128663453 hasConcept C91614233 @default.
- W3128663453 hasConceptScore W3128663453C119599485 @default.