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• W3128965051 endingPage "119952" @default.
• W3128965051 startingPage "119952" @default.
• W3128965051 abstract "Electrochemical ammonia synthesis by N2 fixation has proven to be a promising alternative to the energy-consuming, befouling Haber-Bosch process. Considering the low faradaic efficiency and sluggish kinetics of Nitrogen Reduction Reaction (NRR), it is significant to design a robust and selective catalyst. Herein, we demonstrate a single step in-situ nitridation method to grow cubic molybdenum nitride (γ-Mo2N) nanoparticles on a 2D hexagonal boron nitride (h-BN) sheets as a potential, cost-effective electrocatalyst for NRR, in which the selectivity for N2 was regulated by interfacially engineering the Mo2N-BN bridge. The maneuverability of h-BN sheets enabled the provocation of N-vacancies governed by the particle size, where the fine-tuning of their significance emanated the highest faradaic efficiency of 61.5 %. Moreover, such non-noble metal-based hybrids delivered a stable performance for 20 h. Therefore, our approach of designing the electronic structure of a catalyst by controlling the defects could be an effective practice for selective NRR." @default.
• W3128965051 created "2021-02-15" @default.
• W3128965051 creator A5016663999 @default.
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• W3128965051 date "2021-06-01" @default.
• W3128965051 modified "2023-10-16" @default.
• W3128965051 title "Strong catalyst support interactions in defect-rich γ-Mo2N nanoparticles loaded 2D-h-BN hybrid for highly selective nitrogen reduction reaction" @default.
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• W3128965051 doi "https://doi.org/10.1016/j.apcatb.2021.119952" @default.
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