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• W3129174501 abstract "Abstract Interface segregation of solute atoms has a profound effect on properties of engineering alloys. The occurrence of solute segregation in coherent twin boundaries (CTBs) in Mg alloys is commonly considered to be induced by atomic size effect where solute atoms larger than Mg take extension sites and those smaller ones take compression sites in CTBs. Here we report an unusual solute segregation phenomenon in a group of Mg alloys—solute atoms larger than Mg unexpectedly segregate to compression sites of {10 $$overline 1$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mover> <mml:mrow> <mml:mn>1</mml:mn> </mml:mrow> <mml:mo>¯</mml:mo> </mml:mover> </mml:math> 1} fully coherent twin boundary and do not segregate to the extension or compression site of {10 $$overline 1$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mover> <mml:mrow> <mml:mn>1</mml:mn> </mml:mrow> <mml:mo>¯</mml:mo> </mml:mover> </mml:math> 2} fully coherent twin boundary. We propose that such segregation is dominated by chemical bonding (coordination and solute electronic configuration) rather than elastic strain minimization. We further demonstrate that the chemical bonding factor can also predict the solute segregation phenomena reported previously. Our findings advance the atomic-level understanding of the role of electronic structure in solute segregation in fully coherent twin boundaries, and more broadly grain boundaries, in Mg alloys. They are likely to provide insights into interface boundaries in other metals and alloys of different structures." @default.
• W3129174501 created "2021-02-15" @default.
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• W3129174501 date "2021-02-01" @default.
• W3129174501 modified "2023-10-06" @default.
• W3129174501 title "Unusual solute segregation phenomenon in coherent twin boundaries" @default.
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• W3129174501 doi "https://doi.org/10.1038/s41467-021-21104-8" @default.
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