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• W3129202410 startingPage "152916" @default.
• W3129202410 abstract "The use of a malonate nucleophile in the transition metal-catalyzed hydroalkylation of 1,3-dienes remains immature. Herein, we report the nickel-catalyzed hydroalkylation of 1,3-dienes with malonates using a homoallyl carbonate as the 1,3-diene and hydride source. A broad range of homoally carbonates and malonate derivatives were well tolerated under a Ni/DPEphos catalyst system, providing the corresponding 1,2-hydroalkylation products in 40–94% yields with excellent regioselectivity (32 examples). We also suggested the possible reaction mechanism for the nickel-catalyzed hydroalkylation of in situ generated 1,3-dienes with malonates." @default.
• W3129202410 created "2021-03-01" @default.
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• W3129202410 date "2021-03-01" @default.
• W3129202410 modified "2023-10-18" @default.
• W3129202410 title "Nickel-catalyzed hydroalkylation of 1,3-dienes with malonates using a homoallyl carbonate as the 1,3-diene and hydride source" @default.
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• W3129202410 doi "https://doi.org/10.1016/j.tetlet.2021.152916" @default.
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