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- W3129395567 abstract "Because of their outstanding electrocatalytic activity, M–N–C catalysts have got increasing attention, especially for oxygen reduction reaction (ORR). Nevertheless, M–N–C catalysts still face the great challenges of long-term stability and mass production for practical applications. In this work, we reported the synthesis and study of a honeycomb-like self-supported Co–N–C catalyst, which exhibited desirable activity and excellent stability for ORR in both alkaline and acidic mediums. Specifically, after a 10,000-cycle accelerated durability test, Co–N–C-700 showed a slight decrease of 5 mV in alkaline and no attenuation in acidic solutions for the half-wave potential. The unprecedented ORR performance of the self-supported Co–N–C may be contributed to the unique honeycomb-like morphology, high active surface area, high contents of graphitic N and Co–Nx, and the high intrinsic activity of the Co–Nx moiety. The breakthrough of the highly durable and scalable fabrication of M–N–C catalysts could open a promising way for their potential applications in many fields, including fuel cells and metal–air batteries." @default.
- W3129395567 created "2021-03-01" @default.
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- W3129395567 date "2021-02-19" @default.
- W3129395567 modified "2023-10-17" @default.
- W3129395567 title "Honeycomb-like Self-Supported Co–N–C Catalysts with an Ultrastable Structure: Highly Efficient Electrocatalysts toward Oxygen Reduction Reaction in Alkaline and Acidic Solutions" @default.
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- W3129395567 doi "https://doi.org/10.1021/acsaem.0c03092" @default.
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