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- W3129855684 endingPage "2006135" @default.
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- W3129855684 abstract "Construction of 2D transition metal dichalcogenide (TMD)-based epitaxial heterostructures with different compositions is important for various promising applications, including electronics, photonics, and catalysis. However, the rational design and controlled synthesis of such kind of heterostructures still remain challenge, especially for those consisting of layered TMDs and other non-layered materials. Here, a facile one-pot, wet-chemical method is reported to synthesize Cu2−χSySe1−y-MoS2 heterostructures in which two types of different epitaxial configurations, i.e., vertical and lateral epitaxies, coexist. The chalcogen ratio (S/Se) in Cu2−χSySe1−y and the loading amount of MoS2 in the heterostructures can be tuned. Impressively, the obtained Cu2−χSySe1−y-MoS2 heterostructures can be transformed to CdSySe1−y-MoS2 without morphological change via cation exchange. As a proof-of-concept application, the obtained CdSySe1−y-MoS2 heterostructures with controllable compositions are used as photocatalysts, exhibiting distinctive catalytic activities toward the photocatalytic hydrogen evolution under visible light irradiation. The method paves the way for the synthesis of different TMD-based lateral epitaxial heterostructures with unique properties for various applications." @default.
- W3129855684 created "2021-03-01" @default.
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- W3129855684 date "2021-02-19" @default.
- W3129855684 modified "2023-09-27" @default.
- W3129855684 title "Preparation of CdS <i> <sub>y</sub> </i> Se <sub>1−</sub> <i> <sub>y</sub> </i> ‐MoS <sub>2</sub> Heterostructures via Cation Exchange of Pre‐Epitaxially Synthesized Cu <sub>2−</sub> <i> <sub>χ</sub> </i> S <i> <sub>y</sub> </i> Se <sub>1−</sub> <i> <sub>y</sub> </i> ‐MoS <sub>2</sub> for Photocatalytic Hydrogen Evolution" @default.
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- W3129855684 doi "https://doi.org/10.1002/smll.202006135" @default.
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