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• W3129925304 endingPage "2003469" @default.
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• W3129925304 abstract "Inorganic solid-state electrolyte (SSE) based Na-metal batteries have received extensive attention in next-generation lithium-free energy storage systems with both high-security and superior electrochemical performance. Herein, in contrast to the conventionally used polymer/ceramic/polymer sandwich electrolyte, an efficient green and scalable powder-polishing synthetic method is developed to fabricate a pyrolyzed-polyacrylonitrile modified Na super ionic conductor (NASICON) electrolyte to relieve polarization of integrated composite SSE and ameliorate interfacial contact between the electrolyte and the Na anode. Furthermore, introducing S in the preferable isotropous sulfurized polyacrylonitrile (SPAN) interlayer can trigger dehydrogenation and cyclization of polyacrylonitrile with chemically-bonded short-chain SS segments, which can bond with Na+ to redistribute the interfacial electric field and homogenize transported Na+ flux, leading to transition of Na deposition behavior from dendrite growth mode to lateral flat-shape growth tendency. The conjugated polymer backbones possess delocalized radicals that can activate formed short-chain sulfides to reconnect to the backbones, thus maintaining superior structural stability. Benefiting from the rational interfacial design, a record-high value of 1.4 mA cm−2 for critical current density of Na/SPAN-NASICON/Na cells is obtained. Moreover, SPAN is used as a cathode to assemble solid-state Na/SPAN-NASICON/SPAN Na-organosulfur batteries, demonstrating superior capacity and cycling-stability. The rational SPAN-based structural design strategy may provide an avenue for potential application of solid-state alkali metal batteries." @default.
• W3129925304 created "2021-03-01" @default.
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• W3129925304 date "2021-02-25" @default.
• W3129925304 modified "2023-10-14" @default.
• W3129925304 title "Isotropous Sulfurized Polyacrylonitrile Interlayer with Homogeneous Na⁺Flux Dynamics for Solid‐State Na Metal Batteries" @default.
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• W3129925304 doi "https://doi.org/10.1002/aenm.202003469" @default.
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