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• W3130904208 abstract "We study the bending mode of pure water and charged aqueous surfaces using heterodyne-detected vibrational sum-frequency generation spectroscopy. We observe a low ($1626text{ }text{ }{mathrm{cm}}^{ensuremath{-}1}$) and a high ($1656text{ }text{ }{mathrm{cm}}^{ensuremath{-}1}$) frequency component that can be unambiguously assigned to an interfacial dipole and a bulk quadrupolar response, respectively. We thus demonstrate that probing the bending mode provides structural and quantitative information on both the surface and the bulk." @default.
• W3130904208 created "2021-03-01" @default.
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• W3130904208 date "2021-09-09" @default.
• W3130904208 modified "2023-09-24" @default.
• W3130904208 title "Direct Evidence for a Surface and Bulk Specific Response in the Sum-Frequency Generation Spectrum of the Water Bend Vibration" @default.
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• W3130904208 doi "https://doi.org/10.1103/physrevlett.127.116001" @default.
• W3130904208 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34558941" @default.
• W3130904208 hasPublicationYear "2021" @default.
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