Matches in SemOpenAlex for { <https://semopenalex.org/work/W3130928386> ?p ?o ?g. }
- W3130928386 endingPage "118059" @default.
- W3130928386 startingPage "118059" @default.
- W3130928386 abstract "Abstract Owing to the environmental and technological problems of current commercial homogeneous organometallic catalysts, developing efficient heterogeneous catalysts for ethene dimerization is of industrial importance. Nickel-exchanged zeolite beta (Ni-beta) is a promising catalyst for this reaction due to its highly stable 1-butene yield. Here, we report that the Ni-beta catalyst shows a considerably better 1-butene yield when prepared by solid-state ion exchange compared to liquid-phase ion exchange and incipient wetness impregnation. A combination of CO IR, Ni K-edge X-ray absorption and UV-vis spectroscopies, and density functional theory calculations demonstrate that solid-state ion exchange is an efficient method to form the intrazeolitic mono(μ-oxo)dinickel ([Ni-O-Ni]2+) species which are more active for ethene dimerization than the widely accepted Ni2+ ions." @default.
- W3130928386 created "2021-03-01" @default.
- W3130928386 creator A5050392894 @default.
- W3130928386 creator A5078561388 @default.
- W3130928386 date "2021-04-01" @default.
- W3130928386 modified "2023-10-13" @default.
- W3130928386 title "Ethene dimerization over Ni-beta catalysts prepared by solid-state ion exchange" @default.
- W3130928386 cites W1846217891 @default.
- W3130928386 cites W1973210652 @default.
- W3130928386 cites W1980175885 @default.
- W3130928386 cites W1983304051 @default.
- W3130928386 cites W1987035356 @default.
- W3130928386 cites W1989453627 @default.
- W3130928386 cites W1990643101 @default.
- W3130928386 cites W1993648768 @default.
- W3130928386 cites W1994716441 @default.
- W3130928386 cites W2003162132 @default.
- W3130928386 cites W2008924548 @default.
- W3130928386 cites W2023271753 @default.
- W3130928386 cites W2029280817 @default.
- W3130928386 cites W2044591029 @default.
- W3130928386 cites W2046354949 @default.
- W3130928386 cites W2059052222 @default.
- W3130928386 cites W2061329737 @default.
- W3130928386 cites W2062190443 @default.
- W3130928386 cites W2063534190 @default.
- W3130928386 cites W2070227796 @default.
- W3130928386 cites W2073197754 @default.
- W3130928386 cites W2075626252 @default.
- W3130928386 cites W2084146026 @default.
- W3130928386 cites W2089072035 @default.
- W3130928386 cites W2091540664 @default.
- W3130928386 cites W2092435355 @default.
- W3130928386 cites W2116776591 @default.
- W3130928386 cites W2143765146 @default.
- W3130928386 cites W2230244691 @default.
- W3130928386 cites W2332377568 @default.
- W3130928386 cites W2351343940 @default.
- W3130928386 cites W2562044353 @default.
- W3130928386 cites W2562726782 @default.
- W3130928386 cites W2621507669 @default.
- W3130928386 cites W2791827918 @default.
- W3130928386 cites W2794522566 @default.
- W3130928386 cites W2808458853 @default.
- W3130928386 cites W2876769074 @default.
- W3130928386 cites W2897104891 @default.
- W3130928386 cites W2951153102 @default.
- W3130928386 cites W4242365956 @default.
- W3130928386 doi "https://doi.org/10.1016/j.apcata.2021.118059" @default.
- W3130928386 hasPublicationYear "2021" @default.
- W3130928386 type Work @default.
- W3130928386 sameAs 3130928386 @default.
- W3130928386 citedByCount "11" @default.
- W3130928386 countsByYear W31309283862021 @default.
- W3130928386 countsByYear W31309283862022 @default.
- W3130928386 countsByYear W31309283862023 @default.
- W3130928386 crossrefType "journal-article" @default.
- W3130928386 hasAuthorship W3130928386A5050392894 @default.
- W3130928386 hasAuthorship W3130928386A5078561388 @default.
- W3130928386 hasConcept C107814960 @default.
- W3130928386 hasConcept C117760992 @default.
- W3130928386 hasConcept C127413603 @default.
- W3130928386 hasConcept C145148216 @default.
- W3130928386 hasConcept C147789679 @default.
- W3130928386 hasConcept C161790260 @default.
- W3130928386 hasConcept C178790620 @default.
- W3130928386 hasConcept C185592680 @default.
- W3130928386 hasConcept C192562407 @default.
- W3130928386 hasConcept C199360897 @default.
- W3130928386 hasConcept C2776174256 @default.
- W3130928386 hasConcept C41008148 @default.
- W3130928386 hasConcept C42360764 @default.
- W3130928386 hasConceptScore W3130928386C107814960 @default.
- W3130928386 hasConceptScore W3130928386C117760992 @default.
- W3130928386 hasConceptScore W3130928386C127413603 @default.
- W3130928386 hasConceptScore W3130928386C145148216 @default.
- W3130928386 hasConceptScore W3130928386C147789679 @default.
- W3130928386 hasConceptScore W3130928386C161790260 @default.
- W3130928386 hasConceptScore W3130928386C178790620 @default.
- W3130928386 hasConceptScore W3130928386C185592680 @default.
- W3130928386 hasConceptScore W3130928386C192562407 @default.
- W3130928386 hasConceptScore W3130928386C199360897 @default.
- W3130928386 hasConceptScore W3130928386C2776174256 @default.
- W3130928386 hasConceptScore W3130928386C41008148 @default.
- W3130928386 hasConceptScore W3130928386C42360764 @default.
- W3130928386 hasFunder F4320322120 @default.
- W3130928386 hasLocation W31309283861 @default.
- W3130928386 hasOpenAccess W3130928386 @default.
- W3130928386 hasPrimaryLocation W31309283861 @default.
- W3130928386 hasRelatedWork W2090850713 @default.
- W3130928386 hasRelatedWork W2330924834 @default.
- W3130928386 hasRelatedWork W2331592696 @default.
- W3130928386 hasRelatedWork W2407181204 @default.
- W3130928386 hasRelatedWork W2606102261 @default.
- W3130928386 hasRelatedWork W2726840033 @default.
- W3130928386 hasRelatedWork W2748952813 @default.
- W3130928386 hasRelatedWork W2768655412 @default.
- W3130928386 hasRelatedWork W2899084033 @default.