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- W3131536246 abstract "The evolution of life on earth eventually leads to the emergence of species with increased complexity and diversity. Similarly, evolutionary chemical space exploration in the laboratory is a key step to pursue the structural and functional diversity of supramolecular systems. Here, we present a powerful tool that enables rapid peptide diversification and employ it to expand the chemical space for supramolecular functions. Central to this strategy is the exploitation of palladium-catalyzed Suzuki-Miyaura cross-coupling reactions to direct combinatorial synthesis of peptide arrays in microtiter plates under an open atmosphere. Taking advantage of this in situ library design, our results unambiguously deliver a fertile platform for creating a set of intriguing peptide functions including green fluorescent protein-like peptide emitters with chemically encoded emission colors, hierarchical self-assembly into nano-objects, and macroscopic hydrogels. This work also offers opportunities for quickly surveying the diversified peptide arrays and thereby identifying the structural factors that modulate peptide properties." @default.
- W3131536246 created "2021-03-01" @default.
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- W3131536246 date "2021-02-15" @default.
- W3131536246 modified "2023-10-15" @default.
- W3131536246 title "High-Throughput Peptide Derivatization toward Supramolecular Diversification in Microtiter Plates" @default.
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- W3131536246 doi "https://doi.org/10.1021/acsnano.0c05423" @default.
- W3131536246 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7992134" @default.
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