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- W3131757215 endingPage "152922" @default.
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- W3131757215 abstract "• The BC-rings of canonical SL was constructed by the acid-mediated cascade cyclization. • An 18-hydroxycarlactonoate derivative was successfully converted to rac -4DO/5DS. • The cyclization demonstrated “in flask” may be analogous to that in planta . • The 4π-electrocyclic reaction-based mechanism is proposed. Strigolactones are a group of apocarotenoids known as rhizosphere semiochemicals and phytohormones. Canonical strigolactone consists of a tricyclic lactone (ABC-rings) and a butenolide moiety (D-ring). Although strigolactone biosynthesis has been extensively studied, the process of BC-ring formation has not been elucidated to date. In this study, the chemical conversion of an 18-hydroxycarlactonoate derivative into racemic 4-deoxyorobanchol/5-deoxystrigol was achieved by the acid-mediated cascade cyclization. The acid-mediated BC-ring formation may offer inspiring suggestion for the currently unclear BC-ring formation in strigolactone biosynthesis." @default.
- W3131757215 created "2021-03-01" @default.
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- W3131757215 date "2021-03-01" @default.
- W3131757215 modified "2023-10-03" @default.
- W3131757215 title "Studies on strigolactone BC-ring formation: Chemical conversion of an 18-hydroxycarlactonoate derivative into racemic 4-deoxyorobanchol/5-deoxystrigol via the acid-mediated cascade cyclization" @default.
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- W3131757215 doi "https://doi.org/10.1016/j.tetlet.2021.152922" @default.
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