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- W3131821487 abstract "I present a photon statistics method for quasi-one dimensional sub-diffraction limited nanofluidic motions of single molecules using Feynman-Enderlein path integral approach. The theory is validated in Monte Carlo simulation platform to provide fundamental understandings of Knudsen type flow and diffusion of single molecule fluorescence in liquid. Distribution of single molecule burst size can be precise enough to detect molecular interaction. Realisation of this theoretical study considers several fundamental aspects of single-molecule nanofluidics, such as electrodynamics, photophysics, and multi-molecular events/molecular shot noise. I study two different sizes of molecules, one with 2 nm and another with 20 nm hydrodynamic radii driven by a wide range of flow velocities. The study reports distinctly different velocity dependent nanofluidic regimes, which have not been theoretically as well as experimentally reported earlier. Experimental single-molecule fluorescence bursts inside all-silica nanofluidic channels are used to validate the robustness of the method. It is not restricted to single molecule environment of uniform electrodynamic interactions and can be used to investigate complex refractive index mismatch related non-uniform single-molecule electrodynamic interactions as well. This fundamental investigation of single-molecule nanofluidics has a potential to accelerate the progress of dynamic and complex single-molecule experiments, such as dynamic heterogeneity, biomolecular interactions of misfolded proteins, and nanometric cavity electrodynamics." @default.
- W3131821487 created "2021-03-01" @default.
- W3131821487 creator A5086791315 @default.
- W3131821487 date "2021-02-22" @default.
- W3131821487 modified "2023-09-27" @default.
- W3131821487 title "Feynman-Enderlein Path Integral for Single-Molecule Nanofluidics" @default.
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- W3131821487 hasPublicationYear "2021" @default.
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