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- W3131838596 abstract "We report here on structure-related aggregation effects of short-range ordered aluminosilicates (SROAS) that have to be considered in the development of synthesis protocols and may be relevant for the properties of SROAS in the environment. We synthesized SROAS of variable composition by neutralizing aqueous aluminium chloride with sodium orthosilicate at ambient temperature and pressure. We determined elemental composition, visualized morphology by microscopic techniques, and resolved mineral structure by solid-state 29Si and 27Al nuclear magnetic resonance and Fourier-transform infrared spectroscopy. Nitrogen sorption revealed substantial surface loss of Al-rich SROAS that resembled proto-imogolite formed in soils and sediments due to aggregation upon freezing. The effect was less pronounced in Si-rich SROAS, indicating a structure-dependent effect on spatial arrangement of mass at the submicron scale. Cryomilling efficiently fractured aggregates but did not change the magnitude of specific surface area. Since accessibility of surface functional groups is a prerequisite for sequestration of substances, elucidating physical and chemical processes of aggregation as a function of composition and crystallinity may improve our understanding of the reactivity of SROAS in the environment." @default.
- W3131838596 created "2021-03-01" @default.
- W3131838596 creator A5026853154 @default.
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- W3131838596 date "2021-02-18" @default.
- W3131838596 modified "2023-10-04" @default.
- W3131838596 title "Synthesis of short-range ordered aluminosilicates at ambient conditions" @default.
- W3131838596 cites W1595305358 @default.
- W3131838596 cites W1908259550 @default.
- W3131838596 cites W1965817918 @default.
- W3131838596 cites W1966027316 @default.
- W3131838596 cites W1967249406 @default.
- W3131838596 cites W1968153409 @default.
- W3131838596 cites W1968594531 @default.
- W3131838596 cites W1969472422 @default.
- W3131838596 cites W1979520497 @default.
- W3131838596 cites W1982054526 @default.
- W3131838596 cites W1982471858 @default.
- W3131838596 cites W1983829696 @default.
- W3131838596 cites W1985708982 @default.
- W3131838596 cites W1986239393 @default.
- W3131838596 cites W1987153967 @default.
- W3131838596 cites W1989016472 @default.
- W3131838596 cites W1989999327 @default.
- W3131838596 cites W1990505667 @default.
- W3131838596 cites W1993300057 @default.
- W3131838596 cites W1994630002 @default.
- W3131838596 cites W1997527774 @default.
- W3131838596 cites W1999464010 @default.
- W3131838596 cites W2004072011 @default.
- W3131838596 cites W2005638488 @default.
- W3131838596 cites W2006209334 @default.
- W3131838596 cites W2006553984 @default.
- W3131838596 cites W2009680009 @default.
- W3131838596 cites W2012736794 @default.
- W3131838596 cites W2016175628 @default.
- W3131838596 cites W2017379696 @default.
- W3131838596 cites W2022313166 @default.
- W3131838596 cites W2023788374 @default.
- W3131838596 cites W2024093844 @default.
- W3131838596 cites W2025350325 @default.
- W3131838596 cites W2025708805 @default.
- W3131838596 cites W2025961828 @default.
- W3131838596 cites W2026622888 @default.
- W3131838596 cites W2027241914 @default.
- W3131838596 cites W2031661093 @default.
- W3131838596 cites W2038133973 @default.
- W3131838596 cites W2043112434 @default.
- W3131838596 cites W2045334254 @default.
- W3131838596 cites W2046447185 @default.
- W3131838596 cites W2050445582 @default.
- W3131838596 cites W2055099618 @default.
- W3131838596 cites W2056891847 @default.
- W3131838596 cites W2057794932 @default.
- W3131838596 cites W2060626360 @default.
- W3131838596 cites W2060730218 @default.
- W3131838596 cites W2067099580 @default.
- W3131838596 cites W2068617467 @default.
- W3131838596 cites W2071246550 @default.
- W3131838596 cites W2075045515 @default.
- W3131838596 cites W2081672653 @default.
- W3131838596 cites W2081704598 @default.
- W3131838596 cites W2084233178 @default.
- W3131838596 cites W2087019341 @default.
- W3131838596 cites W2097955508 @default.
- W3131838596 cites W2107502925 @default.
- W3131838596 cites W2109107429 @default.
- W3131838596 cites W2111105585 @default.
- W3131838596 cites W2117350830 @default.
- W3131838596 cites W2117382336 @default.
- W3131838596 cites W2117558441 @default.
- W3131838596 cites W2123996576 @default.
- W3131838596 cites W2131945198 @default.
- W3131838596 cites W2133034835 @default.
- W3131838596 cites W2138300695 @default.
- W3131838596 cites W2139794248 @default.
- W3131838596 cites W2142166808 @default.
- W3131838596 cites W2142888772 @default.
- W3131838596 cites W2147769267 @default.
- W3131838596 cites W2152730208 @default.
- W3131838596 cites W2159707379 @default.
- W3131838596 cites W2163694818 @default.
- W3131838596 cites W2169695809 @default.
- W3131838596 cites W2171602757 @default.
- W3131838596 cites W2281715687 @default.
- W3131838596 cites W2290143139 @default.
- W3131838596 cites W2295554439 @default.
- W3131838596 cites W2335424748 @default.
- W3131838596 cites W2620910387 @default.
- W3131838596 cites W2760402845 @default.
- W3131838596 cites W2796144685 @default.
- W3131838596 cites W2810475051 @default.
- W3131838596 cites W2898788028 @default.
- W3131838596 cites W2914667334 @default.
- W3131838596 cites W3033173864 @default.
- W3131838596 cites W3091076379 @default.