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- W3132155626 abstract "The first metastable phase Ag, ZnS: α-In 2 S 3 QDs were synthesized by ultrafast light-material interaction. The multiple irradiation of millisecond flash pulses facilitated thermodynamic non-equilibrium superheating and quenching for metastable QD formation, as well as sequential self-formation of α-In 2 S 3 QD nucleation, Ag-doping and ZnS-passivation by photo-responsive ionic kinetics. Upon multiple illumination of flash pulses, the synthesis mechanism of Ag, ZnS: α-In 2 S 3 QD was experimentally proved by atomic-resolution transmission electron microscopy (AR-TEM), scanning TEM (STEM) and diverse spectral analysis. To verify the metastable phase QD formation by superheating/quenching in reaction solution, the localized surface plasmon (LSP) properties and instantaneous temperature increment were theoretically calculated using finite-difference time-domain (FDTD) method. Finally, optoelectronic performance and long-term stability of as-synthesized QDs were evaluated by demonstrating the broad wavelength metal-semiconductor-metal (MSM) photoelectric device. • The first ultrafast light-induced metastable quantum dots were synthesized by one-step sequential self-formation. • Upon multiple illumination of flash pulses, synthesis mechanism of Ag, ZnS: α-In2S3 QD was experimentally proved. • The localized surface plasmon properties were theoretically calculated using finite-difference time-domain method. • Optoelectronic performance and long-term stability of QDs were evaluated by demonstrating MSM photoelectric device." @default.
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- W3132155626 date "2021-06-01" @default.
- W3132155626 modified "2023-10-13" @default.
- W3132155626 title "Metastable quantum dot for photoelectric devices via flash-induced one-step sequential self-formation" @default.
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- W3132155626 doi "https://doi.org/10.1016/j.nanoen.2021.105889" @default.
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