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- W3132168993 endingPage "2010499" @default.
- W3132168993 startingPage "2010499" @default.
- W3132168993 abstract "Lithium-sulfur batteries (LSBs) are considered a promising next-generation energy storage device owing to their high theoretical energy density. However, their overall performance is limited by several critical issues such as lithium polysulfide (PS) shuttles, low sulfur utilization, and unstable Li metal anodes. Despite recent huge progress, the electrolyte/sulfur ratio (E/S) used is usually very high (≥20 µL mg−1), which greatly reduces the practical energy density of devices. To push forward LSBs from the lab to the industry, considerable attention is devoted to reducing E/S while ensuring the electrochemical performance. To date, however, few reviews have comprehensively elucidated the possible strategies to achieve that purpose. In this review, recent advances in low E/S cathodes and anodes based on the issues resulting from low E/S and the corresponding solutions are summarized. These will be beneficial for a systematic understanding of the rational design ideas and research trends of low E/S LSBs. In particular, three strategies are proposed for cathodes: preventing PS formation/aggregation to avoid inadequate dissolution, designing multifunctional macroporous networks to address incomplete infiltration, and utilizing an imprison strategy to relieve the adsorption dependence on specific surface area. Finally, the challenges and future prospects for low E/S LSBs are discussed." @default.
- W3132168993 created "2021-03-01" @default.
- W3132168993 creator A5012039029 @default.
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- W3132168993 creator A5071303877 @default.
- W3132168993 creator A5075692415 @default.
- W3132168993 creator A5081328308 @default.
- W3132168993 date "2021-02-23" @default.
- W3132168993 modified "2023-10-14" @default.
- W3132168993 title "Rational Designs for Lithium‐Sulfur Batteries with Low Electrolyte/Sulfur Ratio" @default.
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