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- W3132548319 abstract "Engineering a stable solid electrolyte interphase (SEI) is one of the critical maneuvers in improving the performance of a lithium anode for high-energy-density rechargeable lithium batteries. Herein, we build a fluorinated lithium/sodium hybrid interphase via a facile electroless electrolyte-soaking approach to stabilize the repeated plating/stripping of lithium metal. Jointed experimental and computational characterizations reveal that the fluorinated hybrid SEI mainly consisting of NaF, LiF, LixPOyFz, and organic components features a mosaic polycrystalline structure with enriched grain boundaries and superior interfacial properties toward Li. This LiF/NaF hybrid SEI exhibits improved ionic conductivity and mechanical strength in comparison to the SEI without NaF. Remarkably, the fluorinated hybrid SEI enables an extended dendrite-free cycling of metallic Li over 1300 h at a high areal capacity of 10 mAh cm–2 in symmetrical cells. Furthermore, full cells based on the LiFePO4 cathode and hybrid SEI-protected Li anode sustain long-term stability and good capacity retention (96.70% after 200 cycles) at 0.5 C. This work could provide a new avenue for designing robust multifunctional SEI to upgrade the metallic lithium anode." @default.
- W3132548319 created "2021-03-01" @default.
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- W3132548319 date "2021-02-15" @default.
- W3132548319 modified "2023-10-13" @default.
- W3132548319 title "Electroless Formation of a Fluorinated Li/Na Hybrid Interphase for Robust Lithium Anodes" @default.
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- W3132548319 doi "https://doi.org/10.1021/jacs.0c12051" @default.
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