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• W3132942255 endingPage "100053" @default.
• W3132942255 startingPage "100053" @default.
• W3132942255 abstract "• Recent progress of transition-metal-based materials for alkaline water splitting. • Structure engineering strategies of transition-metal-based materials are highlighted. • Challenges and opportunities of transition-metal-based materials for alkaline water splitting are pointed out. Electrochemical water splitting in alkaline media provides a promising pathway for sustainable hydrogen production that is enssential for a future hydrogen economy . However, the slow reaction rate of hydrogen reaction in alkaline media, and unfavorable kinetics for oxygen evolution reaction have hindered the progress of water splitting technologies for clean hydrogen production. Considering the high price and scarce storage of noble metals which are known as the most effective catalysts for water splitting, it is urgently required to develop non-noble metals based alternatives with highly intrinsic acivity, low price and high tolerance to increase electrocatalytic efficiency and reduce the reaction overpotential from an economic perspective. In this review, we summarize recent research efforts in exploiting advanced transition metal based electrocatalysts with outstanding performance for water splitting catalysis, mainly including transition-metal-based chalcogenides , phosphides, nitrides and carbides as well as single atom catalysts. First, we give a simple description of water splitting mechanism in alkaline media. Then we discuss the promising structural design of transition metal based electrocatalysts for enhancing water splitting, and disclose the underlying relationship between structure and electrocatalytic performance for water splitting with assistance of theoretical simulation. Finally, we provide our personal perspective to highlight the challenges and propose the opportunities for developing transition metal based electrocatalysts for water splitting in alkaline solution. Transition-meta-based materials provide great potential for alkaline water splitting applications. This review summarizes and highlights recent structural design for transition-metal-based electrocatalysts including phosphides, nitrides, chalcogenides and carbides. The electrocatalytic activity-structure relationship ( e.g. , heteroatom doping, defect, interface, single atom engineering) is discussed in details." @default.
• W3132942255 created "2021-03-01" @default.
• W3132942255 creator A5024599426 @default.
• W3132942255 creator A5037493153 @default.
• W3132942255 creator A5082943201 @default.
• W3132942255 date "2021-03-01" @default.
• W3132942255 modified "2023-10-16" @default.
• W3132942255 title "Noble metal-free electrocatalytic materials for water splitting in alkaline electrolyte" @default.
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