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- W3133237451 abstract "Incorporation of foreign elements into the cathode material is broadly adopted by both academia and industry to improve the battery performance. The lack of an in-depth understanding for the underlying mechanism, however, makes it a largely try-and-error process with unsatisfactory efficiency and effectiveness. This is particularly true for the electrochemical reaction kinetics that is heterogeneous over a broad range of length scales and is determined collectively by the cathode’s electronic structure, lattice configuration, and micro-morphology. Here we unveiled a facet-dependent dopant segregation effect in Zr-modified single-crystal LiNi0.6Co0.2Mn0.2O2 cathode. By forming kinetically favored corners on the cathode particles, the presence of a trace amount of Zr critically modulates the mesoscale reaction kinetics. Our findings suggest that a delicately controlled dopant distribution is a viable strategy for designing the next-generation battery cathode with superior structural and chemical robustness." @default.
- W3133237451 created "2021-03-01" @default.
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- W3133237451 date "2021-06-01" @default.
- W3133237451 modified "2023-10-18" @default.
- W3133237451 title "Selective dopant segregation modulates mesoscale reaction kinetics in layered transition metal oxide" @default.
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- W3133237451 doi "https://doi.org/10.1016/j.nanoen.2021.105926" @default.
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