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W3133671353 endingPage "120318" @default.
W3133671353 startingPage "120318" @default.
W3133671353 abstract "This review summarized the synthetic strategies for obtaining the 3d-4f complexes with mixed organic ligands, and the structural and magnetic regulations for this kind of complexes were also provided. • Provide a method for regulating the topologies and magnetism of 3d-4f complexes. • Discuss the mechanisms of the magnetic couplings between different metal ions. • Provide an outlook for further improving the SMM performance of 3d-4f complexes. Since 1993, single molecule magnets (SMMs) have received a wide attention for their potential applications in high-density information storage device, quantum computer and spintronics. Particularly, since a Cu II 2 Tb II 2 complex was found to possess slow magnetic relaxation behavior in 2004, 3d-4f heterometallic complexes are being investigated because they can provide the moderate magnetic couplings between 3d and 4f ions and can provide the significant single-ion magnetic anisotropies of 4f ions, which are in favor of improving SMM performance. Choosing an appropriate organic ligand with ligating atoms linked with 3d and 4f ions simultaneously is a key to synthesize 3d-4f complexes. However, synthesizing 3d-4f complexes by employing two kinds of non-carboxylate organic ligands has received little attention. We believe that the metal core topologies, the magnetic couplings, coordination geometries of 4f ions and the magnetic relaxation behavior of the 3d-4f complexes could be modulated by employing several types of non-carboxylate organic ligands due to the large steric effects between the non-carboxylate organic ligands. Based on the considerations, in recent years, we concentrated on the investigations of the 3d-4f complexes with several types of non-carboxylate organic ligands. In this review, we will present a summary of the 3d-4f complexes reported by us. The studies indicate that the metal core topologies and the magnetic couplings of the obtained 3d-4f complexes were indeed regulated, and most of the complexes possess SMM behavior. Finally, we provided some suggestions to further improve the SMM performance of the 3d-4f complexes." @default.
W3133671353 created "2021-03-15" @default.
W3133671353 creator A5030064573 @default.
W3133671353 creator A5068445612 @default.
W3133671353 creator A5075995463 @default.
W3133671353 creator A5082039677 @default.
W3133671353 date "2021-06-01" @default.
W3133671353 modified "2023-10-18" @default.
W3133671353 title "Recent advances in 3d-4f magnetic complexes with several types of non-carboxylate organic ligands" @default.
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