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• W3133845488 abstract "We report on the low-dimensional magnetic behavior of the series of compounds ${mathrm{NiNb}}_{2ensuremath{-}x}{mathrm{V}}_{x}{mathrm{O}}_{6}$ ($0ensuremath{le}xensuremath{le}2$), with a columbite-type crystal structure stabilized at high pressure and temperature. Based on susceptibility, magnetization, and specific-heat measurements, the system is characterized as presenting quasi-one-dimensional magnetism, with ${mathrm{Ni}}^{2+}$ magnetic moments that can be modeled as Ising spins, placed along zigzag chains in the crystal structure. The low-temperature phase is found to consist of an antiferromagnetic arrangement of ferromagnetic chains, and a metamagnetic transition to uniform ferromagnetic order is observed under magnetic fields slightly above ${ensuremath{mu}}_{0}H=1phantom{rule{4pt}{0ex}}mathrm{T}$. We discuss the effects of substituting vanadium for niobium, maintaining the same crystal structure along the whole series of samples. In particular, the long-range magnetic order, most clearly seen for $x=0$, tends to be suppressed as the vanadium content is increased. The exchange interactions are quantified, revealing that the ferromagnetic intrachain interactions vary from about $7phantom{rule{4pt}{0ex}}mathrm{K}$ for ${mathrm{NiNb}}_{2}{mathrm{O}}_{6}$ to $2phantom{rule{4pt}{0ex}}mathrm{K}$ for ${mathrm{NiV}}_{2}{mathrm{O}}_{6}$, remaining one order of magnitude larger than the mean antiferromagnetic interchain coupling." @default.
• W3133845488 created "2021-03-15" @default.
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• W3133845488 date "2021-03-04" @default.
• W3133845488 modified "2023-10-13" @default.
• W3133845488 title "Quasi-one-dimensional magnetic properties of <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msub><mml:mi>NiNb</mml:mi><mml:mrow><mml:mn>2</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mi mathvariant=normal>V</mml:mi><mml:mi>x</mml:mi></mml:msub><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math> compounds synthesized at high pressure in a nonstandard columbite-type structure" @default.
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• W3133845488 doi "https://doi.org/10.1103/physrevb.103.094409" @default.
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