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- W3134486618 abstract "Widespread commercial adoption of polymer electrolytes for lithium-ion batteries has been hindered by subpar transport properties, namely, ionic conductivities of <1 mS/cm at room temperature and slower Li+ compared to anion transport. The developed polymer and water-in-salt electrolyte demonstrated preferential Li+ transport compared to the anion via pulsed field gradient NMR, acceptable ionic conductivities of >1 mS/cm at 25 °C, and an extended electrochemical stability window compared to water-in-salt electrolytes. This polymer electrolyte has a flexible liquid/solid transition through polymer molecular weight tuning, and both liquid and solid iterations are investigated. MD simulations provided additional insight into the Li+ solvation environment and the mechanism of fast, preferential Li+ transport through percolation of water-rich Li+(H2O)n nanodomains inside the poly(ethylene oxide) matrix." @default.
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- W3134486618 date "2021-03-01" @default.
- W3134486618 modified "2023-10-16" @default.
- W3134486618 title "Water Domain Enabled Transport in Polymer Electrolytes for Lithium-Ion Batteries" @default.
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- W3134486618 doi "https://doi.org/10.1021/acs.macromol.0c01960" @default.
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