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• W3134944539 endingPage "1969" @default.
• W3134944539 startingPage "1962" @default.
• W3134944539 abstract "Abstract The electrochemical reduction of CO 2 (ERC) to valuable chemicals has attracted extensive attention. However, the relatively low selectivity and efficiency of the reaction remain challenges. In this study, Cu electrodes derived from Cu 2 O with predominant (111) facets are synthesized by cetyltrimethylammonium bromide‐assisted preparation. The optimized electrode shows a high faradaic efficiency of 90 % for HCOOH obtained by ERC at −2.0 V (vs.SCE), which surpasses most reported Cu electrodes. Based on a comprehensive analysis of the relationship between the catalytic activity and the thickness of the Cu 2 O layer, the catalytic activity of the unit active site on the Cu 2 O‐derived Cu electrodes is found to be higher than that on the blank Cu electrode. DFT calculations indicate that OCHO* would be produced preferentially over *COOH in the presence of cetyltrimethylammonium bromide (CTAB). This deduction is verified by testing of the effects of CTAB and KBr addition on HCOO − selectivity." @default.
• W3134944539 created "2021-03-15" @default.
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• W3134944539 date "2021-03-18" @default.
• W3134944539 modified "2023-09-23" @default.
• W3134944539 title "Electrochemical Production of Formic Acid from CO ₂ with Cetyltrimethylammonium Bromide‐Assisted Copper‐Based Catalysts" @default.
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• W3134944539 doi "https://doi.org/10.1002/cssc.202100275" @default.
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