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- W3135032232 abstract "Abstract We have measured depletion spectra of the heteronuclear ( 85 Rb 87 Rb + ) dimer cation complexed with up to 10 He atoms. Two absorption bands are observed between 920 and 250 nm. The transition into the repulsive 1 2 Σ u + state of HeRb 2 + gives rise to a broad feature at 790 nm (12,650 cm −1 ); it exhibits a blueshift of 98 cm −1 per added He atom. The transition into the bound 1 2 Π u state of HeRb 2 + reveals vibrational structure with a band head at ≤ 15,522 cm −1 , a harmonic constant of 26 cm −1 , and a spin–orbit splitting of ≤ 183 cm −1 . The band experiences an average redshift of − 38 cm −1 per added He atom. Ab initio calculations rationalize the shape of the spectra and spectral shifts with respect to the number of helium atoms attached. For a higher number of solvating helium atoms, symmetric solvation on both ends of the Rb 2 + ion is predicted." @default.
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- W3135032232 date "2021-03-01" @default.
- W3135032232 modified "2023-10-17" @default.
- W3135032232 title "Electronic transitions in Rb2+ dimers solvated in helium" @default.
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- W3135032232 doi "https://doi.org/10.1007/s00214-021-02728-x" @default.
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