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• W3135114376 abstract "A facile one-step microemulsion method was applied to introduce a Mo promoter into a [email protected] catalyst with a yolk-shell structure ([email protected]). Mo atoms were inserted in the silica shell framework to form SiMoOx species instead of a typical NiMo alloy. It was found that the formation of SiMoOx significantly enhanced the electron-donating ability of Ni sites and the acidity of the support, which improved the methane activation of the catalyst for dry reforming of methane. [email protected] contained the most SiMoOx species and displayed the best catalytic activity and significantly enhanced the TOFCH4 value compared with [email protected] In addition, the oxidation of Ni sites by CO2 was suppressed due to the electron-donating effect of the multivalent molybdenum species in SiMoOx. The [email protected] catalyst displayed favourable stability with WGHSV = 240,000 mL g−1 h−1 compared with undoped [email protected] The formation of NiMo alloy on [email protected] prepared by an impregnation method significantly decreased the catalytic activity." @default.
• W3135114376 created "2021-03-15" @default.
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• W3135114376 date "2021-08-01" @default.
• W3135114376 modified "2023-10-17" @default.
• W3135114376 title "Enhanced performance of xNi@yMo-HSS catalysts for DRM reaction via the formation of a novel SiMoOx species" @default.
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• W3135114376 doi "https://doi.org/10.1016/j.apcatb.2021.120075" @default.
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