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• W3135700018 abstract "One way to induce insulator-to-metal transitions in the spin-orbit Mott insulator ${mathrm{Sr}}_{2}mathrm{Ir}{mathrm{O}}_{4}$ is to substitute iridium with transition metals (Ru, Rh). However, this creates intriguing inhomogeneous metallic states, which cannot be described by a simple doping effect. We detail the electronic structure of the Ru-doped case with angle-resolved photoemission and show that, in contrast to Rh, it cannot be connected to the undoped case by a rigid shift. We further identify bands below ${E}_{F}$ coexisting with the metallic ones that we assign to nonbonding Ir sites. We rationalize the differences between Rh and Ru by a different hybridization with oxygen, which mediates the coupling to Ir and sensitively affects the effective doping. We argue that the spin-orbit coupling does not control either the charge transfer or the transition threshold." @default.
• W3135700018 created "2021-03-15" @default.
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• W3135700018 date "2021-09-03" @default.
• W3135700018 modified "2023-09-27" @default.
• W3135700018 title "Origin of the different electronic structure of Rh- and Ru-doped <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msub><mml:mi>Sr</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:mi>Ir</mml:mi><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml:mn>4</mml:mn></mml:msub></mml:mrow></mml:math>" @default.
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• W3135700018 doi "https://doi.org/10.1103/physrevb.104.l121104" @default.
• W3135700018 hasPublicationYear "2021" @default.
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