FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W3135929356> ?p ?o ?g. }

• W3135929356 endingPage "15278" @default.
• W3135929356 startingPage "15270" @default.
• W3135929356 abstract "Electrocatalytic nitrogen reduction reaction (NRR) represents a promising alternative route for sustainable ammonia synthesis, which currently dominantly relies on the energy-intensive Haber–Bosch process, while it is significantly hampered by the sluggish reaction kinetics due to the short of glorious electrocatalysts. In this work, we report an efficient porous tin heterostructure with intimate dual interfaces for electrosynthesis of ammonia, which exhibits outstanding NRR efficiency with an NH3 yield rate and Faradaic efficiency as high as 30.3 μg h–1mg–1cat and 41.3%, respectively, and excellent stability as well at a low potential of −0.05 V (vs RHE) in 0.1 M Na2SO4 solution under ambient conditions. This matrix value is superior to the analogue Sn-based heterostructures with a single interface and outperforms the currently state-of-the-art Sn-based catalysts. Comprehensive characterizations and theoretical calculations uncovered the formation of the unique intimate dual interfaces in the tin heterostructure promoting the enhancement of the NRR process, which not only effectively exposes more active sites for stronger N2 chemisorption and activation but also accelerates the interfacial electron transfer and reduces the free energy barrier for the rate-determining *N2H formation step, highlighting the importance of the dual interface effect for the design of electrocatalysts in catalysis." @default.
• W3135929356 created "2021-03-29" @default.
• W3135929356 creator A5000648383 @default.
• W3135929356 creator A5031545775 @default.
• W3135929356 creator A5066507894 @default.
• W3135929356 creator A5072645559 @default.
• W3135929356 date "2021-03-26" @default.
• W3135929356 modified "2023-10-16" @default.
• W3135929356 title "Dual Interface-Engineered Tin Heterostructure for Enhanced Ambient Ammonia Electrosynthesis" @default.
• W3135929356 cites W1992258332 @default.
• W3135929356 cites W2128654538 @default.
• W3135929356 cites W2148707525 @default.
• W3135929356 cites W2156809317 @default.
• W3135929356 cites W2173608881 @default.
• W3135929356 cites W2229614381 @default.
• W3135929356 cites W2312983667 @default.
• W3135929356 cites W2325144921 @default.
• W3135929356 cites W2339336236 @default.
• W3135929356 cites W2555698350 @default.
• W3135929356 cites W2560176924 @default.
• W3135929356 cites W2590980665 @default.
• W3135929356 cites W2604354802 @default.
• W3135929356 cites W2767966656 @default.
• W3135929356 cites W2768089236 @default.
• W3135929356 cites W2768334327 @default.
• W3135929356 cites W2790613799 @default.
• W3135929356 cites W2851584547 @default.
• W3135929356 cites W2894805156 @default.
• W3135929356 cites W2896718212 @default.
• W3135929356 cites W2904135604 @default.
• W3135929356 cites W2909267103 @default.
• W3135929356 cites W2910483443 @default.
• W3135929356 cites W2911309755 @default.
• W3135929356 cites W2916158247 @default.
• W3135929356 cites W2916737721 @default.
• W3135929356 cites W2945223387 @default.
• W3135929356 cites W2946199134 @default.
• W3135929356 cites W2954842080 @default.
• W3135929356 cites W2964801156 @default.
• W3135929356 cites W2967340501 @default.
• W3135929356 cites W2969995230 @default.
• W3135929356 cites W2982225284 @default.
• W3135929356 cites W2983005301 @default.
• W3135929356 cites W2995262218 @default.
• W3135929356 cites W3002561092 @default.
• W3135929356 cites W3013090474 @default.
• W3135929356 cites W3014038739 @default.
• W3135929356 cites W3015290904 @default.
• W3135929356 cites W3036559073 @default.
• W3135929356 cites W3043847042 @default.
• W3135929356 cites W3046422472 @default.
• W3135929356 cites W3151267290 @default.
• W3135929356 cites W4239857556 @default.
• W3135929356 cites W4246112865 @default.
• W3135929356 doi "https://doi.org/10.1021/acsami.1c01160" @default.
• W3135929356 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33769776" @default.
• W3135929356 hasPublicationYear "2021" @default.
• W3135929356 type Work @default.
• W3135929356 sameAs 3135929356 @default.
• W3135929356 citedByCount "17" @default.
• W3135929356 countsByYear W31359293562021 @default.
• W3135929356 countsByYear W31359293562022 @default.
• W3135929356 countsByYear W31359293562023 @default.
• W3135929356 crossrefType "journal-article" @default.
• W3135929356 hasAuthorship W3135929356A5000648383 @default.
• W3135929356 hasAuthorship W3135929356A5031545775 @default.
• W3135929356 hasAuthorship W3135929356A5066507894 @default.
• W3135929356 hasAuthorship W3135929356A5072645559 @default.
• W3135929356 hasConcept C127413603 @default.
• W3135929356 hasConcept C130349721 @default.
• W3135929356 hasConcept C134121241 @default.
• W3135929356 hasConcept C147789679 @default.
• W3135929356 hasConcept C161790260 @default.
• W3135929356 hasConcept C171250308 @default.
• W3135929356 hasConcept C17525397 @default.
• W3135929356 hasConcept C178790620 @default.
• W3135929356 hasConcept C181258405 @default.
• W3135929356 hasConcept C185592680 @default.
• W3135929356 hasConcept C191897082 @default.
• W3135929356 hasConcept C192562407 @default.
• W3135929356 hasConcept C193115255 @default.
• W3135929356 hasConcept C2776382133 @default.
• W3135929356 hasConcept C33989665 @default.
• W3135929356 hasConcept C42360764 @default.
• W3135929356 hasConcept C49040817 @default.
• W3135929356 hasConcept C525849907 @default.
• W3135929356 hasConcept C52859227 @default.
• W3135929356 hasConcept C55904794 @default.
• W3135929356 hasConcept C79794668 @default.
• W3135929356 hasConceptScore W3135929356C127413603 @default.
• W3135929356 hasConceptScore W3135929356C130349721 @default.
• W3135929356 hasConceptScore W3135929356C134121241 @default.
• W3135929356 hasConceptScore W3135929356C147789679 @default.
• W3135929356 hasConceptScore W3135929356C161790260 @default.
• W3135929356 hasConceptScore W3135929356C171250308 @default.
• W3135929356 hasConceptScore W3135929356C17525397 @default.
• W3135929356 hasConceptScore W3135929356C178790620 @default.
• W3135929356 hasConceptScore W3135929356C181258405 @default.

• next