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• W3136016132 endingPage "1167" @default.
• W3136016132 startingPage "1159" @default.
• W3136016132 abstract "Preparing green materials with excellent performance based on coordination chemistry is a challenge. In the present work, a new energetic complex, [Co(Hatzc)2(H2O)2] · 2H2O (1) (H2atzc = 3-carboxyl-5-amino-1,2,4-triazole), was synthesized by the diffusion method and characterized by X-ray single-crystal diffraction, elemental analysis, infrared spectral analysis, and thermogravimetric analysis. The structural analyses illustrate that 1 exhibits a 0-D motif, linked by hydrogen-bonding interactions to give a 3-D supramolecular architecture. 1 shows good thermal stability (Tdec =283 °C), low sensitivity (IS > 40J, FS > 360N), prominent detonation velocity (10.18 km s−1), and detonation pressure (44.99 Gp). The heat of detonation of 1 (4.109 kcal g−1) is higher than most classical energetic complexes as shown by density functional theory (DFT). In addition, 1 shows good catalytic activity toward AP (ammonium perchlorate) decomposition by thermodynamics and dynamic analysis, which indicates 1 is a potential energetic candidate in the solid propellant field." @default.
• W3136016132 created "2021-03-29" @default.
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• W3136016132 date "2021-03-03" @default.
• W3136016132 modified "2023-10-18" @default.
• W3136016132 title "A new oxygen-rich and poly-nitrogen energetic complex: synthesis, properties of high energy materials and catalytic decomposition of ammonium perchlorate" @default.
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• W3136016132 doi "https://doi.org/10.1080/00958972.2021.1892663" @default.
• W3136016132 hasPublicationYear "2021" @default.
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