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- W3136097145 abstract "Introducing oxygen vacancy (Vo) has been considered as an effective and significant method to accelerate the sluggish electrocatalytic nitrogen reduction reaction (NRR). In this work, a series of bimetallic zeolitic imidazolate frameworks based on ZIF-67 and ZIF-8 with varied ratios of Co/Zn have been applied as precursors to prepare Vo-rich Zn-doped Co3O4 nanopolyhedrons (Zn–Co3O4) by a low-temperature oxidation strategy. Zn–Co3O4 presents an ammonia yield of 22.71 μg h–1 mgcat.–1 with a high faradaic efficiency of 11.9% for NRR under ambient conditions. The remarkable catalytic performances are believed to result from the plentiful Vo as the Lewis acid sites and electron-rich Co sites to promote the adsorption and dissociation of N2 molecules. Remarkably, Zn–Co3O4 also demonstrates a high electrochemical stability. This work presents a guiding method for developing a stable and efficient electrocatalyst for the NRR." @default.
- W3136097145 created "2021-03-29" @default.
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- W3136097145 date "2021-03-18" @default.
- W3136097145 modified "2023-10-07" @default.
- W3136097145 title "Oxygen Vacancy Engineering of MOF-Derived Zn-Doped Co<sub>3</sub>O<sub>4</sub> Nanopolyhedrons for Enhanced Electrochemical Nitrogen Fixation" @default.
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- W3136097145 doi "https://doi.org/10.1021/acsami.0c22767" @default.
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