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- W3136134841 abstract "Colloidal quantum dot (QD) materials are promising candidates for luminescent solar concentrator (LSC) technology thanks to their broadband absorption above semiconductor bandgap and tunable Stokes-shift for minimizing the light reabsorption. Previously reported QDs in LSC contain non-polar organic ligands that can be easily incorporated into common host matrix/waveguide materials – polyacrylates or polycarbonates, however, these organic ligands on QD surfaces introduce problems when some new matrix materials are employed. For example, cellulose nanocrystal (CNC), a wood-derived eco-friendly material, has the potential for LSC, but no solvents are available to dissolve both QD and CNC simultaneously. Here we report high-quality luminescent films employing QD-CNC hybrid materials. Such films are produced from stable QD-CNC suspension by applying solution-phase exchange to replace non-polar organic ligands on QDs to the metal halide complex, as well as performing acetylation on CNC surfaces. The fabricated QD-CNC hybrid film keeps similar photoluminescence quantum yield and lifetime compared to as-synthesized QDs in non-polar organic solvents. The developed method in this work has the potential to be widely used to mix QD with other materials having polar functional groups." @default.
- W3136134841 created "2021-03-29" @default.
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- W3136134841 date "2021-07-01" @default.
- W3136134841 modified "2023-10-16" @default.
- W3136134841 title "Luminescent films employing quantum dot-cellulose nanocrystal hybrid nanomaterials" @default.
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- W3136134841 doi "https://doi.org/10.1016/j.matlet.2021.129737" @default.
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