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• W3136161840 endingPage "138155" @default.
• W3136161840 startingPage "138155" @default.
• W3136161840 abstract "In this study, we report the use of reactive binding strategy to fix carbon-based oxygen reduction reaction (ORR) catalyst to metal current collector for the first time. Reactive binder, e.g. phenol-formaldehyde resin (PFR) oligomer, is developed as an alternative to the popularly used Nafion binder to bond carbon-based ORR catalyst, e.g. Pt/C (Pt loaded on VulcanX C72R carbon black), onto stainless steel (SS) current collector for use as cathode in microbial fuel cells. The ORR electrocatalytic performance of the Pt/C electrode bonded by PFR (Pt/C-PFR) is studied in neutral medium and compare with that bonded by the Nafion binder (Pt/C-Nafion). Results show that the dosage of PFR binder in the Pt/C-PFR could be only half that of Nafion binder in the Pt/C-Nafion, and the resulted Pt/C-PFR shows superior ORR electrocatalytic performance and stability to that of Pt/C-Nafion on the SS current collector. A strong interaction is developed between the SS and the PFR binder, which is four times of that between the SS and the Nafion binder. X-ray photoelectron spectroscopy results reveal that the higher bonding strength can be attributed to the formation of C−O−Fe bonds between the PFR and the SS. This study offers a low-cost and effective binding strategy for generating high-performance and scalable ORR electrode." @default.
• W3136161840 created "2021-03-29" @default.
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• W3136161840 date "2021-06-01" @default.
• W3136161840 modified "2023-10-16" @default.
• W3136161840 title "The use of reactive binder for carbon-based oxygen reduction reaction catalyst in neutral medium" @default.
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• W3136161840 doi "https://doi.org/10.1016/j.electacta.2021.138155" @default.
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